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解沛忠课题组在Green Chem.发表研究论文
阅读次数: 添加时间:2021/08/23 发布:

Dehydrative allylation of P-H species under metal-free conditions

Xiaobo Yang,a Bowen Li,a Huicong Xing,a Ju Qiu,a Teck-Peng Loh,ab and Peizhong Xiea*

a School of Chemistry and Molecular Engineering, Nanjing Tech University, Nanjing 211816, P. R. China.

b Division of Chemistry and Biological Chemistry, School of Physical and Mathematical Sciences, Nanyang Technological University, Singapore 637371.

Abstract: An environmentally benign protocol for C-P bond construction was developed under metal- and solvent-free conditions. In the presence of B(C6F5)3, wide-spectrum P-H species, including dialkylphosphite, hypophosphite ester, and secondary phosphine oxides, can be successfully incorporated into the dehydrative cross-coupling process with allylic alcohols delivering the corresponding allylic organophosphorus compounds in high yields.

Green Chem. 2021, 23, 1633-1637.(影响因子:10.182

论文链接:https://pubs.rsc.org/en/content/articlepdf/2021/gc/d1gc00191d

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